IADR Abstract Archives

An Amphiphilic Dendritic Molecule as a Template for Apatite Crystalization

Objective: Biomimetic mineral-polymer composites are of great interest for their many applications, such as cell culture medium, scaffolds for hard tissue engineering and templates for mineralization. The purpose of this study is to synthesize a novel material based on dendritic molecules with functional amino acid as the building blocks, by which to regulate the crystallization of apatite (AP) in liquid environment.

Materials and Methods: The Poly (amino amine) dendrons were synthesized and further modified with aspartic acid on the periphery and an aliphatic chain at the focal point (Sa-BM2-Asp). Sa-BM2-Asp was dissolved in dimethyl sulfoxide (DMSO) at the concentration of 10-3mol 20ìL and then dropped into the aqueous solution with calcium nitrate and diammonium hydrogen phosphate. The aggregation of Sa-BM2-Asp was confirmed by transmission electron microscopy (TEM), and crystals of AP developed with the assemblies from Sa-BM2-Asp as the template. The features of the obtained composite were determined by XRD, FT-IR, HRTEM and SEM.

Results: The aggregates of Sa-BM2-Asp were observed by TEM with the diameter around 15-35nm. FT-IR measurement was performed to characterize the structure of the deposition that was the crystals of AP. Moreover, the crystals of AP showed fiber-like morphology. XRD result provided that the growth of the crystals was along with the direction of (002).

Conclusion: The newly synthesized amphiphilic dendritic molecule could self-assemble in aqueous solution. It would act as a template for the mineralization, leading to the orientation development of apatite.


Division: IADR/AADR/CADR General Session
Meeting: 2011 IADR/AADR/CADR General Session (San Diego, California)
Location: San Diego, California
Year: 2011
Final Presentation ID: 1957
Abstract Category|Abstract Category(s): Dental Materials 6: Polymer-based Materials-Chemistry and Composition
Authors
  • Yang, Sheng  ( Peking University School and Hospital of Stomatology, Beijing, N/A, China )
  • Wang, Lei  ( Peking University, Beijing P.R.C, N/A, China )
  • He, Hai  ( Beijing National Laboratory for Molecular Sciences, and Key Laboratory of Polymer Chemistry and Physics of the Ministry of Educa, Beijing, N/A, China )
  • Jia, Xinru  ( Beijing National Laboratory for Molecular Sciences, and Key Laboratory of Polymer Chemistry and Physics of the Ministry of Educa, Beijing, N/A, China )
  • Feng, Hailan  ( Peking University School and Hospital of Stomatology, Beijing, N/A, China )
  • SESSION INFORMATION
    Poster Session
    New Materials, Modified Materials and Materials Characterization
    03/18/2011