IADR Abstract Archives

X-Ray Photoelectron Spectroscopy Characterization of Six Dentin Bonding Agents

Objective: This study analyzed the chemical composition of the first 10nm of the external layer of six dentin bonding agents using X-ray Photoelectron Spectroscopy (XPS). The goal was to compare the surface composition of adhesives from two different generations.

Method: Adper Easy Bond (AEB), Adper Prompt L-Pop (APL), Xeno III (XE3) Xeno IV (XE4), iBond Self Etch (ISE), and iBond Total Etch (ITE) samples were prepared and polymerized according to the supplier’s instructions with a Light-Emitting Diode unit (Ultradent- 750 mW). The samples (n=3) were analyzed by XPS (Kratos Axis, vacuum of 2x10-9 torr, an x-ray gun emission set to 15 mA, and an x-ray gun anode HT set to 15 kV, which equates to a power setting of 225 W).  XPS surveys and high-resolution scans were taken from the external layer (depth = 0nm, (D0)) and a sub-surface layer (depth = 10nm, (D10)) after removing the external surface with Argon etching. Carbon (C1s) (at 285 eV) and Oxygen (O1s) peaks were used to compare the deconvolution of the peaks.

Result: 1) XPS survey: Statistically significant differences (p<0.05) of C1s and O1s percentages were found between D0 and D10 for all adhesives. Also, at D0: C1s for AEB and APL (80.85±0.91; 61.95±1.31), O1s for XE3 and XE4 (27.5±0.72; 7.75±1.2), and for ISE and ITE (11.89±0.42; 3.93±0.34) showed significant differences. 2) XPS high resolution: All adhesives displayed contributions from carbon impurities for C1s at 285 eV at D0, but not at D10. 

Conclusion: All adhesives in this study showed that their atomic compositions in the external layer were not uniform, and their compositions, in the thickness probed, varied with depth from the surface.

Division: IADR/AADR/CADR General Session
Meeting: 2013 IADR/AADR/CADR General Session (Seattle, Washington)
Location: Seattle, Washington
Year: 2013
Final Presentation ID: 1874
Abstract Category|Abstract Category(s): Dental Materials 2: Adhesion - Leakage/Margin Assessments
Authors
  • Robertson, Lindsay  ( University of Manitoba, Winnipeg, MB, Canada )
  • Gong, Victor  ( University of Manitoba, Winnipeg, MB, Canada )
  • Pesun, Igor  ( University of Manitoba, Winnipeg, MB, Canada )
  • França, Rodrigo  ( University of Manitoba, Winnipeg, MB, Canada )
  • SESSION INFORMATION
    Poster Session
    Adhesion - Leakage/Margin Assessments I
    03/22/2013